Building a "convertible double action Ruger" really isn't as hard as most people think. Sure, there are a lot of moving parts that need to fall in line (well, not really a lot), but the likelihood that they do is high, and the consequence if they don't is low.
I've done it successfully 3 times to make 45colt dedicated and 454Casull dedicated convertible Redhawks or convert a 45colt to 454C (and 454c to 45colt, which I resold at huge markdown), as well as a recent one where I made a convertible 357mag & 357/44 Mag Redhawk.
[C]an I buy a 357 cylinder and crane complete assembly and install it with minimal to no fitting on my security six?
Yes, you can, but you MIGHT have to try a couple of times to find a proper cylinder that fits (might - don't count on it).
The guys here are right - they have to line up for lock up, headspace, and b/c gap. That sounds like a lot that has to line up, but it pretty commonly does.
The good news is that you'll only be out about $10 for shipping if it doesn't fit. Most Ruger parts DO fit interchangeably, with the lowest risk coming from specimen from the same production era. If you buy a new cylinder and it doesn't fit, then you can easily resell it for what you paid for it, so you're just out the shipping. Minimum risk.
You will need to get a range rod to be able ensure alignment, and of course, feeler gauges to check out headspace and B/C gap.
You can save yourself some time/trouble if you measure out your current revolver to determine your "ideal" specs and your tolerable range of specs, then compare that to the take-off cylinder. But not everybody will do that - if you want it, buy it, if not, I'll sell it to someone else.
So yes - go buy a cylinder & crane assy, try it out. If it fits for all critical dimensions, send it out and get it reamed. If not, sell it and try again.